@Ultragorgon9
I actually did think a lot about the supporting characters, but I widened the selection of Britt's allies: Lenore Case and Mike Axford are obvious mainstays, but I also want to see the "forgotten" Daily Sentinel characters Jasper Jenks and Ed Lowry (from the radio series and the '40s film serials). Showing who they are would give the audience a good taste of what the people of Century City (which I'm using here as a placeholder for whatever city this Green Hornet works in, though it could actually be Century like in the Dynamite comics) are like, since our only references otherwise are three white Americans (this number goes down depending on how Irish Mike is portrayed) and one Asian immigrant.
The only actor who comes to my mind for Lenore Case is Alicia Witt, who recently starred in the horror movie Longlegs. She has the red hair that Wende Wagner made an iconic part of Miss Case's appearance in the 1966 show, and even though she's over 40 years old, she doesn't look older than the previous actresses who played Miss Case, Wagner and Anne Nagel (the latter from the film serials).
Alan Tudyk would be my pick for Michael Axford. He's been in everything and has incredible acting experience, and he looks quite similar to Lloyd Gough (the actor who played Axford in the TV show). He's played several characters with the same kind of mania that Mike always has when he thinks the Hornet is involved, like Harry in Resident Alien or Wat in A Knight's Tale. He's also old enough that the original backstory of starting as a cop and becoming a news reporter makes sense; you can't have Axford played by someone in their physical prime, because then he'd still be on the police force.
I don't know who should play Jasper Jenks or Ed Lowry, but I think there should only be one of them. Jenks was, after all, created as a replacement for Mike Axford. Lowry seems like the best fit for this role, given his distinguishing feature as the Sentinel's young star reporter. Ed Lowry and Mike Axford would make for a good comic relief duo, given that the rest of the cast would be more in line with the dark detective crime drama that I hope the movie will be.
You might have noticed that I didn't include everyone's favourite district attorney on my list of supporting characters I want in this movie. That's because Frank Scanlon works with an experienced Green Hornet, and I expect this movie to be the origin story of the Green Hornet. In the same way that only a veteran Batman has Robin, Britt Reid wouldn't start working with Scanlon as soon as he becomes a vigilante. I think the movie should end with the Green Hornet and D.A. Scanlon becoming allies, showing how Britt has grown into the role.
This ties into my overall ideas about how the plot should go, though, which is that Britt Reid develops throughout the story into the expert crimefighter we see in the 1966 show. He would start the movie with just himself, Kato, Kato's souped-up armored car (later fully converted into the Black Beauty), and the gas gun. The elaborate Hornet's Nest base, the Hornet Sting, and Scanlon all are gradually brought in. In the same line of thinking, I think Britt should reveal his secret identity to Lenore Case near the end of the story, as a bit of a nod to how she knows his identity in the TV show but not in most earlier works (e.g., the film serials).
On the topic of the Green Hornet's rogues gallery, though... definitely the most recognisable is the Black Hornet from Kevin Smith's Britt Reid Jr. comics, but for a Green Hornet movie starting with the expectation that the audience doesn't know about the original Green Hornet, he's unusable. My personal favourites have to be (in no particular order) the Firebug from the TV episode "The Hornet and the Firefly", Low Singh and his martial arts gang from the episode "The Preying Mantis", Peter Eden from the two-parter episode "Beautiful Dreamer", and Mr. Bordine and Stella Merja from the 1941 serial The Green Hornet Strikes Again!
I think Mr. Bordine and Stella Merja work best as villains for a Green Hornet "year one" style movie. They both work for the mob, unlike my other favourite rogues, but they're more interesting than other ordinary crooks. Bordine is an experienced racketeer enforcer with scars all over his face, giving him some built-in menace; I suggest turning him into a psychotic hired gun, kind of like the Daredevil villain Bullseye, or perhaps more like Two-Face in Batman: The Animated Series. Ms. Merja, meanwhile, can disguise herself as other people through clever makeup usage and a wig; in a more amped-up superhero movie, this could instead be some kind of sci-fi technology (like the Spider-Man villain Chameleon). For a more pulpy science fiction villain angle, her face itself could be malleable like wax, allowing her to reshape it entirely. I don't know who to cast as Ms. Merja, but I could absolutely see Michael Wincott playing Bordine. He's got the sociopathic demeanor for it.
Also, if we get any costumed villains similar to the fake Green Hornet gang in the TV episode "Crime Wave", who dress up like the Hornet either to pin the blame on him or to gain notoriety with their own secret identity, they should be led by a crime boss played by Seth Rogen. It would fit him well.